unshackle verb2 •To remove shackles from someone or something.The captain ordered that the guards unshackle and release the prisoner, as he had served his sentence. •To remove restrictions or inhibitions; to allow full freedom and power.Painting was, as it were, a new art, and being unshackled by old models it chose its own subjects, and took an eagle’s flight. — 1818 formsunshackled · unshackling · unshackles