unsettled adjective4 •Not in a steady condition, uncertain, subject to change. •Disturbed, upset.I was unsettled by the sudden outburst, and since I didn't know what to do I just stood there, confused. •Not populated, having no settlers or other inhabitants. •Unpaid.We need to settle this bill; even if you think the charge is too high we can't just leave it unsettled. formsmore unsettled · most unsettled