unbound /ʌnˈbaʊnd/ adjective5 •Not bound. •Not tied up.The hostages' hands were left unbound. •Without a binding.an unbound book •Not obligated.The terms of the contract inadvertently left certain unbound aspects to subjective interpretation. •Lying beyond the proton or neutron drip line; having a negative particle separation energy; capable of decaying by the spontaneous exothermic emission of one or more nucleons.Helium-2 is unbound, as it is energetically favorable for it to split into two separate protons.